Stuart A. Rice's Advances in Chemical Physics, Volume 129 PDF

By Stuart A. Rice

ISBN-10: 0471445274

ISBN-13: 9780471445272

This sequence offers the chemical physics box with a discussion board for serious, authoritative reviews of advances in each quarter of the self-discipline. quantity 129 within the sequence maintains to document contemporary advances with major, up to date chapters via across the world famous researchers.

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37. PFPE Zdol 3D simulation results: J=kB T ¼ 1, A=kB T ¼ 1000, K0 =kB T ¼ 4, W0 =kB T ¼ 4, d ! 1, 105 lattice steps. Here, Df is the fractal dimension, which differs for the monolayer and multilayer situations, implying that Df is determined not only by lateral movement (virtually independent of layer thickness) but also by a cascade effect from overlying layers. By quantifying Df as a function of the molecule/surface coupling, as well as the number of monolayers, Df can be used as a fingerprint to analyze lubricant/surface pairs, and possibly become a critical parameter for the selection of optimal lubricants.

104] observed that the iso-free-volume viscosities of Zdol were linearly proportional to MW above their glass transition temperatures. In contrast, we observed a crossover behavior for ZdolTX possessing bulky endgroups. Crossover behavior has been reported for the molecular weight dependence on viscosity for PFPEs with bulky endgroups [105,106]. The existence of an MC in ZdolTX data is similar to the reptation processes normally found in high-molecular-weight polymers, which may arise from strong endgroup interactions by forming a ‘‘temporal tube’’-like confinement.

Kuhn and Kuhn [114] also obtained an expression for intrinsic viscosity for the full range of particle aspect ratio (p) by taking an approach similar to Simha’s method. 645). 455), implying that the apparent shape of the PFPE is ‘‘nonspherical’’ and suggesting the existence of cluster formations. 25. kH values are strongly dependent on the solvent quality, indicating significant differences between the interaction among the ‘‘clusters’’ of PFPE molecules. This cluster formation in solution (or changes in aspect ratio) is related to the dispersion quality of the PFPE (see Fig.

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Advances in Chemical Physics, Volume 129 by Stuart A. Rice


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